Yttrium iron garnet (YIG) is a promising material for various terahertz applications due to its special optical properties. At present, a high-quality YIG wafer is the desire of terahertz communities and it is still challenging to prepare substrate-free YIG single crystal films. In this work, we prepared wafer-level substrate-free La:YIG single crystal films, for the first time, to our knowledge. Terahertz optical and magneto-optical properties of La:YIG films were characterized by terahertz time domain spectroscopy (THz-TDS). Results show that the as-prepared La:YIG film has an insertion loss of less than 3 dB and a low absorption coefficient of less than 10cm-1 below 1.6 THz. Benefitting from the thickness of the substrate-free YIG films and low insertion loss, their terahertz properties could be further manipulated by simply using a wafer-stacking technique. When four La:YIG films were stacked, there was an insertion loss of less than 10 dB in the range of 0.1-1.2THz. The Faraday rotation angle of the four-layer-stacked La:YIG films reached 19°, and the isolation could reach 17 dB. By further increasing the stacking number to eight pieces, a remarkable Faraday rotation angle of 45° was achieved with an isolation of 23 dB, which is important for practical application in the THz band. This material may provide a milestone opportunity to make various non-reciprocal devices, such as isolators and phase shifters.

Metalenses are essential components in terahertz imaging systems. However, without careful design, they show limited field of view and their practical applications are hindered. Here, a wide-angle metalens is proposed whose structure is optimized for focusing within the incident angles of ±25°. Simulation and experiment results show that the focusing efficiency, spot size, and modulation transfer function of this lens are not sensitive to the incident angle. More importantly, this wide-angle metalens follows the ideal Gaussian formula for the object-image relation, which ensures a wider field of view and better contrast in the imaging experiment.

Chiral metasurfaces integrated with active materials can dynamically control the chirality of electromagnetic waves, making them highly significant in physics, chemistry, and biology. Herein, we theoretically proposed a general and feasible design scheme to develop a chiral metadevice based on a bilayer anisotropic metasurface and a monolayer liquid crystal (LC), which can construct and flexibly manipulate arbitrary terahertz (THz) chirality. When the twist angle between the anisotropic axes of two metasurfaces θ is not 0°, the spatial mirror symmetry of the chiral metadevice is broken, resulting in a strong THz chiral response. In addition, the introduction of anisotropic LCs not only enhances the chiral response of the metadevice but also induces the flipping modulation and frequency tunability of the chirality. More importantly, by optimizing the θ, we can flexibly design the arbitrary chiral response and the operating frequency of chirality, thereby promoting the emergence of various chiral manipulation devices. The experimental results show that the maximum circular dichroism can reach -33dB at 0.94 THz and flip to 28 dB at 0.69 THz by rotating the LC optical axis from the x to y axis, with the maximum operating frequency tunable range of ∼120GHz. We expect this design strategy can create new possibilities for the advancement of active THz chiral devices and their applications, including chiral spectroscopy, molecular recognition, biosensing, and fingerprint detection.

Dynamic beam steering with unlimited angular range and fast speed remains a challenge in the terahertz gap, which is urgently needed for next-generation target tracking, wireless communications, and imaging applications. Different from metasurface phased arrays with element-level phase control, here we steer the beam by globally engineering the diffraction of two cascaded metagratings during in-plane rotation. Benefiting from large-angle diffraction and flexible on/off control of the diffraction channels, a pair of metagratings with optimized supercells and proper orientation successfully directs the incoming beam towards any arbitrary direction over the transmission half space, with the steering speed improved more than twice that of the small-angle diffractive designs. Single-beam and dual-beam steering within the solid angle of 1.56π and elevation angle of ±77° has been demonstrated with average throughput efficiency of 41.4% at 0.14 THz, which can be generalized to multiple-beam cases. The dual diffraction engineering scheme offers a clear physical picture for beamforming and greatly simplifies the device structure, with additional merits of large aperture and low power consumption.

Active terahertz (THz) beam manipulation is urgently needed for applications in wireless communication, radar detection, and remote sensing. In this work, we demonstrate a liquid crystal (LC) integrated Pancharatnam–Berry (PB) metadevice for active THz beam manipulation. Through theoretical analysis and simulation design, the geometric phase of the PB metasurface is engineered to match the tunable anisotropic phase shift of LCs under an external magnetic field, and dynamic beam deflection accompanied by spin conversion is obtained. The experimental results show that the device realizes a dynamic modulation depth of >94% and maximum efficiency of over 50% for the different spin states. Moreover, due to the broadband operating characteristics of devices at 0.7–1.3 THz, the deflection angles are frequency dependent with a scanning range of over ±20° to ±32.5°. Moreover, the two conjugate spin states are always spatially separated in different deflection directions with an isolation degree of over 10 dB. Therefore, this metadevice provides a scheme of active THz beam deflection and spin state conversion, and it also achieves both controllable wavelength division multiplexing and spin division multiplexing, which have important potential in large-capacity THz wireless communication.

To enhance and actively control terahertz (THz) anisotropy and chirality, we have designed and fabricated a THz composite device with a liquid crystal (LC) layer and Si anisotropic metasurface. By initial anchoring and electrically rotating the spatial orientation of the LC optical axis, the different symmetry relationships are obtained in this hybrid device. When the optical axis of LC is parallel or perpendicular to the optical axis of the Si metasurface, the anisotropy of the device will be enhanced or offset, which leads to a tunable phase-shift range of more than 180°. When there is an angle between the two optical axes, due to the destruction of the mirror symmetry in the LC-Si anisotropic medium, the highest circular dichroism of the device reaches 30 dB in the middle orientation state of the LC optical axis, and the active modulation can be realized by changing the bias electric field on the LC layer. This composite device demonstrates rich characteristics for the feasible manipulation of THz polarization conversion and chiral transmission, which can be applied in THz polarization imaging and chiral spectroscopy.

The powerful wavefront manipulation capability of metasurfaces originates from their subwavelength or deep subwavelength elements with designable optical responses, especially phase responses. However, they usually suffer from performance degradation as the spatial phase gradient is large. To solve this issue, we propose an accurate and efficient nonlocal diffraction engineering mechanism to tailor an arbitrary large-gradient wavefront utilizing superwavelength-scale elements. The fast-varying phase profile is cut into segments according to 2π zones rather than subwavelength discretization. Each phase segment is accurately implemented by precisely tailoring the diffraction pattern of the element, where diffraction angles, efficiencies, and phases are controlled simultaneously. As proof of the concept, high numerical aperture cylindrical metalenses are designed using this method and experimentally validated at the terahertz band. The cylindrical metalens is further extended to a full-space metalens, which enables high-quality subwavelength imaging with resolved details of 0.65λ. The proposed mechanism offers an efficient way to capture the fast-varying wavefront using relatively coarse geometries with new physical insights.